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1255139
Merging nonlinear acoustics and nonlinear optics : laser generated intense acoustic pulses and breakdown in dielectrics
Christos Flytzanis
Ecole Normale Superieure, Laboratoire Pierre Aigrain, Paris, France
Nonlinear acoustics and nonlinear optics share some common features at the
same time as they markedly differ in others. Both rely on anharmonic wave
couplings but nature has been far more generous with acoustic anharmonicities
than with optical ones and to such an extent that the nonlinear interactions and
propagation of the former ones effectively appear as local while the later show
predominantly nonlocal features.
This is strikingly evidenced in the vastly different space and time scales
involved in the two classes of nonlinear wave generation and propagation and the
underlying mechanisms. Precisely these differences in anharmonicity and
nonlocality shape the opto-acoustic interactions as well and the
amplitude-coherence transfers from the ones to the others, this being
exclusively done from optical to acoustical.
Here we review the optoacoustic processes that lead to large amplitude acoustic
phonon pulse generation in dielectrics using nonlinear electro-optical processes
in the nanosecond-subpicosecond pulse regime.
We first consider the parametric generation of sound pulses without optical
absorption losses and briefly review the use of coherent processes such as
stimulated and impulsive Brillouin effects and phonon and polarization echos to
develop nonlinear acoustic spectroscopy along the same lines as in nonlinear
optical spectroscopy and obtain information about coupling constants of acoustic
waves with other material excitations, relaxation processes and phase
transitions in dielectrics.
We then consider the case of acoustic shock waves generated concomitant with
breakdown and permanent lattice modifications in well confined spots in the
dielectric intermediated through “hot spot” or plasma creation and subsequent
phonon generation and avalanche through anharmonic couplings. The main steps
leading to laser induced breakdown are assessed and analysed and some
applications are briefly presented.
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